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We weren't able to find "uncalm"
Perhaps, you want to check one of these:
uncalm (not calm)
unclasp (to release the clasp of)
unclad (not dressed)
unclamp (to release from a clamp)
unclench (to release or relax a clenched or tight grip)
unclear (not clear or easily understood)
unclutter (to remove clutter or disorder from)